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Hansen et al. Microstructures 2023;3:2023029  https://dx.doi.org/10.20517/microstructures.2023.17  Page 9 of 17

               Table 2. Euclidean, Cosine, and SSIM similarity values compared to the reference pattern, along with the reliability values, in the VO
                                                                                                         2
               on sapphire sample
                Diffraction pattern                                       Similarity method
                                                        Euclidean            Cosine          SSIM
                A                                       0.707                0.841           0.045
                B                                       0.632                0.807           0.046
                C                                       0.678                0.804           0.033
                D                                       0.421                0.771           0.035
                Reliability                             1.043                1.042           1.022



               Table 3. Euclidean, Cosine, and SSIM similarity values compared to the reference pattern, along with the reliability values, in the VO
                                                                                                         2
               on sapphire sample denoised with a Gaussian filter applied (radius = 5)
                Diffraction pattern                                       Similarity method
                                                        Euclidean            Cosine          SSIM
                A                                       0.910                0.919           0.846
                B                                       0.600                0.907           0.666
                C                                       0.723                0.903           0.718
                D                                       0.412                0.284           0.276
                Reliability                             1.259                1.013           1.178
















                Figure 5. Crystallographic variant maps of the VO  thin film on sapphire sample generated using the (A) Euclidean distance, (B) Cosine,
                                                 2
                and (C) SSIM algorithms.




















                Figure 6. VBF image of VO  thin film on sapphire (left) and the selected diffraction patterns (right) after Gaussian filtering (radius = 5)
                                 2
                for similarity quantification.

               variants are very different from the Ref pattern (similarity values are 0.600 and 0.723). The difference is the
               largest when comparing the vacuum diffraction pattern with the Ref pattern, which yields a similarity value
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