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Feng et al. Chem Synth 2023;3:37  https://dx.doi.org/10.20517/cs.2023.26        Page 13 of 16

               Table 1. Comparison of the currently available synthetic strategies toward 2DMMs
                Methods                   Advantages                                   Disadvantages
                Molecular self-assembly method   Controllable preparation;             Strict reaction conditions
                                          Easy removal of templates without residue
                Single micelle assembly method  Precise synthesis control;             Poor crystallinity
                                          Open pore structure
                Multi templates method    Well design and control the mesostructure and 2D morphology  Wide pore size distribution
                                          Diverse accessible surfactants and precursors;   Complex operation
                Surface-limited co-assembly method   Strong universality
                Template free method      Simple and general                           Disordered mesopores

               2D: Two-dimensional; 2DMMs: two-dimensional mesoporous materials.


               components will be developed, the designed preparation of 2D mesoporous heterostructures and
               composites will open up an unknown new design space for material science. Thirdly, 2DMMs are expected
               to make breakthroughs in applications such as membrane separation, catalysis, energy storage, solar cells,
               electronic devices, etc. However, their manufacturing in the future still needs to expand in scale. Therefore,
               in order to meet the needs of industry or commercialization, it is also crucial to prepare high-quality
               2DMMs on a large scale and at a low cost.


               DECLARATIONS
               Authors’ contributions
               Prepared and revised the manuscript: Feng D
               Revised the manuscript: Li X, Zhang L
               Designed and revised the manuscript: Qiao ZA
               All authors contributed to the discussion and preparation of the manuscript.

               Availability of data and materials
               Not applicable.

               Financial support and sponsorship
               This work was supported by the National Natural Science Foundation of China (22105033, 21621001, and
               21671073), the Science and Technology Department of Jilin Province (YDZJ202201ZYTS330 and
               YDZJ202101ZYTS137), the “111” Project of the Ministry of Education of China (B17020), and Program for
               JLU Science and Technology Innovative Research Team, Interdisciplinary Integration and Innovation
               Project of Jilin University.


               Conflicts of interest
               All authors declared that there are no conflicts of interest.


               Ethical approval and consent to participate
               Not applicable.


               Consent for publication
               Not applicable.


               Copyright
               © The Author(s) 2023.
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